CSpace  > 大气环境研究中心
Particulate matter pollution over China and the effects of control policies
Wang, Jiandong1,2; Zhao, Bin3; Wang, Shuxiao1,2; Yang, Fumo4,5; Xing, Jia1,2; Morawska, Lidia6; Ding, Aijun7; Kulmala, Markku8; Kerminen, Veli-Matti8; Kujansuu, Joni8
2017-04-15
摘要

China is one of the regions with highest PM(2.5)concentration in the world. In this study, we review the spatio-temporal distribution of PM2.5 mass concentration and components in China and the effect of control measures on PM2.5 concentrations. Annual averaged PM2.5 concentrations in Central-Eastern China reached over 100 mu g m(-3), in some regions even over 150 mu g m(-3). In 2013, only 4.1% of the cities attained the annual average standard of 35 mu g m(-3). Aitken mode particles tend to dominate the total particle number concentration. Depending on the location and time of the year, new particle formation (NPF) has been observed to take place between about 10 and 60% of the days. In most locations, NPF was less frequent at high PM mass loadings. The secondary inorganic particles (i.e., sulfate, nitrate and ammonium) ranked the highest fraction among the PM2.5 species, followed by organic matters (OM), crustal species and element carbon (EC), which accounted for 6-50%, 15-51%, 5-41% and 2-12% of PM2.5, respectively. In response to serious particulate matter pollution, China has taken aggressive steps to improve air quality in the last decade. As a result, the national emissions of primary PM2.5, sulfur dioxide (SO2), and nitrogen oxides (NOx) have been decreasing since 2005, 2006, and 2011, respectively. The emission control policies implemented in the last decade could result in noticeable reduction in PM2,(5)concentrations, contributing to the decreasing PM2.5 trends observed in Beijing, Shanghai, and Guangzhou. However, the control policies issued before 2010 are insufficient to improve PM2.5 air quality notably in future. An optimal mix of energy-saving and end-of-pipe control measures should be implemented, more ambitious control policies for NMVOC and NH3 should be enforced, and special control measures in winter should be applied. 40-70% emissions should be cut off to attain PM2.5 standard. (C) 2017 Elsevier B.V.All rights reserved.

关键词Pm2.5 Metropolitan Regions Chemical Speciation Control Policies China
DOI10.1016/j.scitotenv.2017.01.027
发表期刊SCIENCE OF THE TOTAL ENVIRONMENT
ISSN0048-9697
卷号584页码:426-447
收录类别SCI
WOS记录号WOS:000399358500042
语种英语